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大气污染 5

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Temporal variation of heavy metal pollution in urban stormwater runoff

Wen LI, Zhenyao SHEN, Tian TIAN, Ruimin LIU, Jiali QIU

《环境科学与工程前沿（英文）》 2012年 第6卷 第5期   页码 692-700 doi: 10.1007/s11783-012-0444-5

摘要： Stormwater runoff from three types of urban surfaces, a parking lot, a street, and a building roof, was monitored during four rainfall events that occurred in the one-year period from June 2009 to June 2010. The event mean concentrations (EMC) of dissolved copper (Cu), lead (Pb), zinc (Zn), manganese (Mn), and iron (Fe) exceeded China’s National Water Quality Standards for Surface Water. The degree of heavy metal contamination was related to the type of underlying surfaces. Additionally, the concentration of dissolved heavy metals peaked shortly after the runoff began and then declined sharply as a result of adequate flushing. First flush effects of varying degrees were also observed during all of the monitored rainfall events based on the first flush ratio ( ). Redundancy analysis revealed that four environmental variables (rainfall depth, intensity, antecedent dry weather period and type of underlying surface) had significant effects on the strengths of the first flush effects, accounting for 72.9% of the variation in the . Dissolved metals presented varying first flush effects on different underlying surfaces that occurred in the following relative order: parking lot>roof>road for low intensity and high runoff volume rainfall events; parking lot>road>roof for high intensity and low runoff volume events. The relative strength of the first flush for dissolved heavy metals was Fe, Mn>Cu, Zn>Pb.

关键词： urban stormwater     heavy metal pollution     temporal variation     event mean concentration     first flush effect     redundancy analysis    

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Plant diversity reduces the effect of multiple heavy metal pollution on soil enzyme activities and microbial

Yang GAO, Chiyuan MIAO, Jun XIA, Liang MAO, Yafeng WANG, Pei ZHOU

《环境科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 213-223 doi: 10.1007/s11783-011-0345-z

摘要： It is unclear whether certain plant species and plant diversity could reduce the impacts of multiple heavy metal pollution on soil microbial structure and soil enzyme activities. Random amplified polymorphic DNA (RAPD) was used to analyze the genetic diversity and microbial similarity in planted and unplanted soil under combined cadmium (Cd) and lead (Pb) pollution. A metal hyperaccumulator, , and a common plant, , were used in this research. The results showed that microorganism quantity in planted soil significantly increased, compared with that in unplanted soil with Cd and Pb pollution. The order of microbial community sensitivity in response to Cd and Pb stress was as follows: actinomycetes>bacteria>fungi. Respiration, phosphatase, urease and dehydrogenase activity were significantly inhibited due to Cd and Pb stress. Compared with unplanted soil, planted soils have frequently been reported to have higher rates of microbial activity due to the presence of additional surfaces for microbial colonization and organic compounds released by the plant roots. Two coexisting plants could increase microbe population and the activity of phosphatases, dehydrogenases and, in particular, ureases. Soil enzyme activity was higher in phytoremediated soil than in planted soil in this study. Heavy metal pollution decreased the richness of the soil microbial community, but plant diversity increased DNA sequence diversity and maintained DNA sequence diversity at high levels. The genetic polymorphism under heavy metal stress was higher in phytoremediated soil than in planted soil.

关键词： enzyme activity     soil DNA     microbial population     plant diversity     heavy metal    

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Evaluating heavy metal contamination of riverine sediment cores in different land-use areas

Wenzhong Tang, Liu Sun, Limin Shu, Chuang Wang

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1283-4

摘要： Abstract • Metal pollution was studied in riverine sediments from different land-use areas. • Cd was the most serious heavy metal contaminant in riverine sediment cores. • Riverine sediment cores from industrial area were most polluted by heavy metals. • B1 fraction determined metal pollution, risk and toxicity in riverine sediments. Anthropogenic activities are regarded as the main sources of heavy metal pollution, yet few studies have investigated the effects of land-use setting on heavy metal accumulation in riverine sediments. Based on both total contents and geochemical fractions, heavy metal pollution, risk and toxicity were determined in riverine sediment cores from different land-use areas (mountain area- MA, farm area- FA, city area- CA, and industrial area- IA) of the Yang River Basin in North China. The results showed that FA had higher contents of riverine sedimentary Cu; CA had higher contents of Cd; IA had higher contents of both Cd and Zn. Most riverine sediments from FA and IA were contaminated with the investigated metals, although these concentrations were evaluated to have low potential ecological risk and no toxicity to benthic organisms. However, a high proportion of Cd in the B1 fraction of riverine sediments in IA indicating high risk should receive more attention. The B1 fraction largely determined the contamination, risk and toxicity levels associated with heavy metals in the riverine sediments of the Yang River Basin.

关键词： Heavy metals     Riverine sediments     Pollution     Land-use    

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基于主成分综合模型的矿区农田重金属污染评价

王从陆,吴超,段瑜

《中国工程科学》 2008年 第10卷 第7期   页码 180-183

摘要：

文章尝试利用变量聚类分析方法对矿区附近农田土壤重金属污染的主要污染物进行辨识，并采用 综合主成分分析法对矿区附近农田土壤重金属污染情况进行评价和分级。分析结果表明：利用变量聚类分 析法可以有效地辨识矿区附近农田土壤重金属污染中的主要成分；运用综合主成分分析法，确定样本的综合 主成分，并对其排序和聚类，可以有效揭示矿区附近农田土壤重金属污染物的数据结构、相互关系和不同样 品点的污染程度。采用主成分分析方法对矿区附近农田土壤重金属污染情况的评价结果，反映了矿区主要 重金属污染物的影响，同时又定量化了土壤复合重金属污染研究。辨识和评价结果可为矿区附近农田土壤 重金属污染治理对策的提出和重点治理区域的确定提供参考和指导。

关键词： 主成分综合模型     矿区农田土壤     重金属污染     评价    

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重金属废水处理技术概述

刘敏敏,于水利,侯立安

《中国工程科学》 2014年 第16卷 第7期   页码 100-105

摘要：

水体重金属污染正成为全世界最严重的环境问题之一，多种多样的技术已被用于重金属废水的处理。本文综述了近年来用于重金属废水处理的常见工艺，包括化学沉淀法、混凝-絮凝、电化学法、膜分离、离子交换法和吸附法等，并对相关工艺进行了评述。

关键词： 重金属废水     膜分离     离子交换     吸附    

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长江三角洲地区农用地土壤重金属污染状况与防治建议

甘婷婷,赵南京,殷高方,马明俊,孟德硕,方丽,杨瑞芳,刘文清

《中国工程科学》 2021年 第23卷 第1期   页码 174-184 doi: 10.15302/J-SSCAE-2021.01.024

摘要：

长江三角洲地区（简称长三角地区）是我国重要的工农业生产基地，关注该地区农用地土壤重金属污染状况对促进地区经济社会良性发展、保障生态环境安全具有重要意义。本文根据近 20 年发表的长三角地区农用地土壤重金属相关文献中的重金属含量数据，全面分析长三角不同区域农用地土壤典型重金属累积情况与污染状况，系统探究导致长三角地区农用地土壤重金属累积与污染的主要原因。分析发现，工业“三废”排放、交通运输、化肥、农药、农膜等的大量施用（使用），使得长三角地区农用地土壤中重金属 Cd 累积与污染情况最为严重，其次是 Cu、 Hg 和 Pb，而浙江台州和安徽铜陵分别存在Cd、 Hg 和 Cu， Cd、 Pb 和 Cu 多种重金属复合污染问题。针对长三角地区农用地土壤重金属污染防治的迫切需求和主要污染成因，在农用地土壤重金属污染源头控制、农用地土壤重金属快速动态监测、农用地土壤分级管理、重金属污染农用地土壤修复新技术研发、农用地土壤污染防治立法等方面提出了相关防治建议，以期为改善长三角地区农用地土壤生态环境、促进优质高效农业的可持续发展提供参考。

关键词： 农用地     重金属     污染     防治     长三角地区    

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Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

《环境科学与工程前沿（英文）》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1091-x

摘要：

Ratio of turbidity and TSS (Tur/TSS) was used to characterize PSD of stormwater particles.

Pb and Zn preferred to accumulate in finer RDS, while Cu, Cr and Ni in coarser RDS.

HMs pollution in stormwater particles increased linearly with Tur/TSS.

Dissolvability of HMs and PSD variations contribute to the differences between RDS and stormwater.

关键词： Road-deposited sediment     Stormwater runoff     Heavy metal     Particle size     Pollution variation    

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Recent progress in electrospun nanofibers and their applications in heavy metal wastewater treatment

《化学科学与工程前沿（英文）》 2023年 第17卷 第3期   页码 249-275 doi: 10.1007/s11705-022-2245-0

摘要： Novel adsorbents with a simple preparation process and large capacity for removing highly toxic and nondegradable heavy metals from water have drawn the attention of researchers. Electrospun nanofiber membranes usually have the advantages of large specific surface areas and high porosity and allowing flexible control and easy functionalization. These membranes show remarkable application potential in the field of heavy metal wastewater treatment. In this paper, the electrospinning technologies, process types, and the structures and types of nanofibers that can be prepared are reviewed, and the relationships among process, structure and properties are discussed. On one hand, based on the different components of electrospun nanofibers, the use of organic, inorganic and organic−inorganic nanofiber membrane adsorbents in heavy metal wastewater treatment are introduced, and their advantages and future development are summarized and prospected. On the other hand, based on the microstructure and overall structure of the nanofiber membrane, the recent progresses of electrospun functional membranes for heavy metal removal are reviewed, and the advantages of different structures for applications are concluded. Overall, this study lays the foundation for future research aiming to provide more novel structured adsorbents.

关键词： electrospinning     heavy metal     adsorption     nanostructure     wastewater    

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Strategies to manage the risk of heavy metal(loid) contamination in agricultural soils

Fang-Jie ZHAO

《农业科学与工程前沿（英文）》 2020年 第7卷 第3期   页码 333-338 doi: 10.15302/J-FASE-2020335

摘要：

Soil contamination with heavy metal(loid)s threatens soil ecological functions, water quality and food safety; the latter is the focus of this review. Cadmium (Cd) and arsenic (As) are the toxic elements of most concern for food safety because they are relatively easily taken up by food crops. Rice is a major contributor of both Cd and As intakes to the Chinese population. Contamination and soil acidification are the main causes of high Cd levels in rice grains produced in some areas of southern China. The risk of Cd and As accumulation in food crops can be mitigated through agronomic practices and crop breeding. Liming is effective and economical at reducing Cd uptake by rice in acid soils. Paddy water management can produce opposite effects on Cd and As accumulation. Many genes controlling Cd and As uptake and translocation have been characterized, paving the way to breeding low accumulating crop cultivars through marker-assisted molecular breeding or genetic engineering. It is important to protect agricultural soils from future contamination. Long-term monitoring of anthropogenic additions and accumulation of heavy metal(loid)s in agricultural soils should be undertaken. Mass-balance models should be constructed to evaluate future trends of metal(loid)s in agricultural soils at a regional scale.

关键词： arsenic     cadmium     food safety     heavy metals     soil contamination    

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Sulfur mediated heavy metal biogeochemical cycles in coastal wetlands: From sediments, rhizosphere to

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1523-x

摘要：

• In sediments, the transformation of sulfides may lead to the release of heavy metals.

关键词： Coastal wetland     Heavy metal     Sulfur     Biogeochemical cycle    

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Nutrient status and pollution levels in five areas around a manganese mine in southern China

Kehui Liu, Xiaolu Liang, Chunming Li, Fangming Yu, Yi Li

《环境科学与工程前沿（英文）》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1279-0

摘要： Abstract • The soil TP level was high or extremely high in all areas. • TN, OM and available Cu were insufficient in EA, TA and RA. • All areas reached the heavily polluted level and had high ecological risk levels. • Mn and Cd were the dominant pollutants. Nutrient status and pollution levels are the main factors affecting soil restoration. The nutrient status and pollution levels in five areas, an unexplored mine area (UA), an explored mine area (EA), a tailings area (TA), a reclamation area (RA) and an agricultural area (AA), around the Pingle manganese mine in Guangxi, China, were assessed in this study. The results showed that the average total phosphorus in these five areas ranged from 1.05 to 1.57 mg/kg, corresponding to grades of extremely high and high. The average total nitrogen values were 0.19, 0.69, 0.93, 1.24 and 1.67 mg/kg in EA, TA, RA, UA and AA, corresponding to grades of very low, low, medium-low, medium-high and medium-high, respectively. The average organic matter values were 12.78, 8.92, 22.77, 21.29 and 29.11 mg/kg in EA, TA, RA, UA and AA, which corresponded to grades of medium-low, low, medium-high, medium-high and medium-high, respectively. All these results indicated that the total phosphorus was sufficient in these areas, while the total nitrogen and organic matter were insufficient in EA, TA and RA. The available concentrations of Mn and Zn corresponded to the intermediate grade, while the values for Cu corresponded to the very low grade; these might be another factor restricting ecological reclamation. Contamination and ecological risk assessments based on the single contamination index, Nemerow multi-factor index and potential ecological risk index showed that the five tested areas around the Mn mine were considered heavily polluted and presented high ecological risk. Mn and Cd were the dominant pollutants.

关键词： Ecological reclamation     Ecological risk assessment     Heavy metal     Mn mine     Soil nutrients    

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A 50-year sedimentary record of heavy metals and their chemical speciations in the Shuangtaizi Riverestuary (China): implications for pollution and biodegradation

Baolin LIU, Ke HU, Zhenglong JIANG, Fengge QU, Xin SU

《环境科学与工程前沿（英文）》 2011年 第5卷 第3期   页码 435-444 doi: 10.1007/s11783-011-0352-0

摘要： Two parallel sediment cores collected from tidal flat located in the Shuangtaizi River estuary were analyzed for heavy metal concentrations and chemical speciations. Based on the Cs activity profile, mean sedimentation rate at the sampling site during the past 50 years was estimated to be 1.3 cm·a . Correlation analyses show that almost all the metals are associated with each other, suggesting that these metals might be derived from same sources and/or affected by same geochemical processes. Influence of total organic carbon (TOC) content on the concentrations of Cr, Ni, Cu and Cd is evident. Silt and clay contents, instead of sand content, play an important role in the distribution of these metals. The dominant binding phases for most of the metals (except for Cd) are the residual. The relative decrease of the residual fraction of Cd and Pb in the upper 66 cm of the core is striking. The distribution of chemical fraction confirms that the residual fractions of these metals have a natural origin, while only the non-residual fractions of Cd and Pb increased upward the core due to pollution in the past five decades. Pollution assessment on these heavy metals based on Index of Geoaccumulation ( ) also demonstrates that most of the metals are unpolluted. The weak pollution as observed in the sediments is perhaps related to a local plant, the Kitag, which may have played a significant role in the biodegradation of these metals and the metal distribution in the estuary.

关键词： Shuangtaizi River estuary     sediment core     heavy metals     pollution    

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Reuse of heavy metal-accumulating

Dongdong MA,Hongwen GAO

《环境科学与工程前沿（英文）》 2014年 第8卷 第6期   页码 952-959 doi: 10.1007/s11783-013-0619-8

摘要： Phytoremediation technology is regarded as a simple and efficient way to remove heavy metals from contaminated soil. A reasonable disposal of metal hyperaccumulators is always a major issue in waste reuse and resource-saving. The heavy metal-accumulating (L.) was investigated where heavy metals were desorbed by a facile acid-treatment. The result indicated that more than 90% of heavy metals (Zn, Pb and Cu) was extracted from with 0.2 mmol·L HCl. The plant residue was used to adsorb heavy metals ions. The adsorption fitted the Langmuir isotherm model with the saturation adsorption capacity of 9.5 mg·g Zn , 36.2 mg·g Pb and 12.9 mg·g Cu , and the surface complexation and the backfilling of heavy metal-imprinting cavities existed simultaneously during the adsorption. The treatment of wastewaters indicated that the plant residue exhibited a high removal rate of 97% for Cu. Also, the material could be recycled. The method offers a new disposal approach for heavy metal hyperaccumulator.

关键词： heavy metals     Cynondon dactylon     acid-treatment     adsorption     recycling    

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Nanoscale Zero-Valent Iron (nZVI) for Heavy Metal Wastewater Treatment: A Perspective

Shaolin Li,Lei Li,Weixian Zhang,

《工程（英文）》 doi: 10.1016/j.eng.2023.08.012

摘要： Industries such as non-ferrous metal smelting discharge billions of gallons of highly toxic heavy metal wastewater (HMW) worldwide annually, posing a severe challenge to conventional wastewater treatment plants and harming the environment. HMW is traditionally treated via chemical precipitation using lime, caustic, or sulfide, but the effluents do not meet the increasingly stringent discharge standards. This issue has spurred an increase in research and the development of innovative treatment technologies, among which those using nanoparticles receive particular interest. Among such initiatives, treatment using nanoscale zero-valent iron (nZVI) is one of the best developed. While nZVI is already well known for its site-remediation use, this perspective highlights its application in HMW treatment with metal recovery. We demonstrate several advantages of nZVI in this wastewater application, including its multifunctionality in sequestrating a wide array of metal(loid)s (> 30 species); its capability to capture and enrich metal(loid)s at low concentrations (with a removal capacity reaching 500 mg·g–1 nZVI); and its operational convenience due to its unique hydrodynamics. All these advantages are attributable to nZVI’s diminutive nanoparticle size and/or its unique iron chemistry. We also present the first engineering practice of this application, which has treated millions of cubic meters of HMW and recovered tons of valuable metals (e.g., Cu and Au). It is concluded that nZVI is a potent reagent for treating HMW and that nZVI technology provides an eco-solution to this toxic waste.

关键词： Nanoscale zero-valent iron     Wastewater     Heavy metal     Resource recovery    

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EFFECT OF EXOGENOUS ADDITIVES ON HEAVY METAL PASSIVATION AND NITROGEN RETENTION IN PIG MANURE COMPOSTING

《农业科学与工程前沿（英文）》 doi: 10.15302/J-FASE-2023487

摘要：

● Research on heavy metal passivation and nitrogen emissions is necessary for the pig industry.

关键词： additives     composting     heavy metals passivation     nitrogen retention     pig manure    

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标题 作者 时间 类型 操作

Temporal variation of heavy metal pollution in urban stormwater runoff

Wen LI, Zhenyao SHEN, Tian TIAN, Ruimin LIU, Jiali QIU

期刊论文

Plant diversity reduces the effect of multiple heavy metal pollution on soil enzyme activities and microbial

Yang GAO, Chiyuan MIAO, Jun XIA, Liang MAO, Yafeng WANG, Pei ZHOU

期刊论文

Evaluating heavy metal contamination of riverine sediment cores in different land-use areas

Wenzhong Tang, Liu Sun, Limin Shu, Chuang Wang

期刊论文

基于主成分综合模型的矿区农田重金属污染评价

王从陆,吴超,段瑜

期刊论文

重金属废水处理技术概述

刘敏敏,于水利,侯立安

期刊论文

长江三角洲地区农用地土壤重金属污染状况与防治建议

甘婷婷,赵南京,殷高方,马明俊,孟德硕,方丽,杨瑞芳,刘文清

期刊论文

Transferral of HMs pollution from road-deposited sediments to stormwater runoff during transport processes

Qian Wang, Qionghua Zhang, Mawuli Dzakpasu, Nini Chang, Xiaochang Wang

期刊论文

Recent progress in electrospun nanofibers and their applications in heavy metal wastewater treatment

期刊论文

Strategies to manage the risk of heavy metal(loid) contamination in agricultural soils

Fang-Jie ZHAO

期刊论文

Sulfur mediated heavy metal biogeochemical cycles in coastal wetlands: From sediments, rhizosphere to

期刊论文

Nutrient status and pollution levels in five areas around a manganese mine in southern China

Kehui Liu, Xiaolu Liang, Chunming Li, Fangming Yu, Yi Li

期刊论文

A 50-year sedimentary record of heavy metals and their chemical speciations in the Shuangtaizi Riverestuary (China): implications for pollution and biodegradation

Baolin LIU, Ke HU, Zhenglong JIANG, Fengge QU, Xin SU

期刊论文

Reuse of heavy metal-accumulating

Dongdong MA,Hongwen GAO

期刊论文

Nanoscale Zero-Valent Iron (nZVI) for Heavy Metal Wastewater Treatment: A Perspective

Shaolin Li,Lei Li,Weixian Zhang,

期刊论文

EFFECT OF EXOGENOUS ADDITIVES ON HEAVY METAL PASSIVATION AND NITROGEN RETENTION IN PIG MANURE COMPOSTING

期刊论文